New chemo-enzymatic route for the synthesis of chiral glycidyl esters ((S)-ethyl and (S)-methyl-4,5-epoxypentanoates) from renewable resources

Title
New chemo-enzymatic route for the synthesis of chiral glycidyl esters ((S)-ethyl and (S)-methyl-4,5-epoxypentanoates) from renewable resources
Publication Date
2016-08-18
Author(s)
Peru, Aurélien
Flourat, Amandine
Duncan, Anthony
Raverty, Warwick
Greatrex, Ben
( author )
OrcID: https://orcid.org/0000-0002-0356-4966
Email: bgreatre@une.edu.au
UNE Id une-id:bgreatre
Allais, Florent
Type of document
Conference Publication
Language
en
Entity Type
Publication
Publisher
American Chemical Society
Place of publication
United States of America
UNE publication id
une:1959.11/60119
Abstract

Chiral glycidyl esters – such as (S)-ethyl- or (S)-methyl-4,5-epoxypentanoates - are valuable precursors in many chemical syntheses. Until recently, these compounds were synthesized from glutamic acid in four steps (deamination, reduction, tosylation and epoxide formation) in low to average global yield (20-50%). Moreover, this procedure requires some harmful reagents such as sodium nitrite (toxic and ecotoxic) and boron hydride (carcinogen).

Herein, to access these chiral glycidyl esters, we propose a safer chemo-enzymatic synthetic pathway starting from levoglucosenone (aka LGO, CAS 37112-31-5), a biobased compound obtained through the flash pyrolysis of cellulose. Firstly, LGO was submitted to a lipase-mediated Baeyer-Villiger oxidation followed by an acidic hydrolysis to afford (S)-γ-hydroxymethyl-α,β-butenolide. The latter then underwent a palladium-catalyzed hydrogenation to give (S)-γ-hydroxymethyl-γ-butyrolactone. Finally, after tosylation, the corresponding intermediate was treated with sodium ethoxide/methoxide to afford (S)-Ethyl and (S)-Methyl-4,5-epoxypentanoates in 57% yield, respectively.

Link
Citation
252nd American Chemical Society National Meeting and Exposition, Chemistry of People, by the People, for the People, v.252
ISSN
0065-7727

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